Aspect's experiment

Aspect's experiment was the first quantum mechanics experiment to demonstrate the violation of Bell's inequalities with photons using distant detectors. Its 1982 result allowed for further validation of the quantum entanglement and locality principles. It also offered an experimental answer to Albert Einstein, Boris Podolsky, and Nathan Rosen's paradox which had been proposed about fifty years earlier.

It was the first experiment to remove the locality loophole, as it was able to modify the angle of the polarizers while the photons were in flight, faster than what light would take to reach the other polarizer, removing the possibility of communications between detectors.

The experiment was led by French physicist Alain Aspect at the Institut d'optique théorique et appliquée in Orsay between 1980 and 1982. Its importance was immediately recognized by the scientific community. Although the methodology carried out by Aspect presents a potential flaw, the detection loophole, his result is considered decisive and led to numerous other experiments (the so-called Bell tests) which confirmed Aspect's original experiment.

For his work on this topic, Aspect was awarded part of the 2022 Nobel Prize in Physics.

Entanglement and the EPR paradox
The Einstein–Podolsky–Rosen (EPR) paradox is a thought experiment proposed by physicists Albert Einstein, Boris Podolsky and Nathan Rosen which argues that the description of physical reality provided by quantum mechanics is incomplete. In the 1935 EPR paper titled "Can Quantum-Mechanical Description of Physical Reality be Considered Complete?", they argued for the existence of "elements of reality" that were not part of quantum theory, and speculated that it should be possible to construct a theory containing these hidden variables. Resolutions of the paradox have important implications for the interpretation of quantum mechanics.

The thought experiment involves a pair of particles prepared in what would later become known as an entangled state. Einstein, Podolsky, and Rosen pointed out that, in this state, if the position of the first particle were measured, the result of measuring the position of the second particle could be predicted. If instead the momentum of the first particle were measured, then the result of measuring the momentum of the second particle could be predicted. They argued that no action taken on the first particle could instantaneously affect the other, since this would involve information being transmitted faster than light, which is forbidden by the theory of relativity. They invoked a principle, later known as the "EPR criterion of reality", positing that: "If, without in any way disturbing a system, we can predict with certainty (i.e., with probability equal to unity) the value of a physical quantity, then there exists an element of reality corresponding to that quantity." From this, they inferred that the second particle must have a definite value of both position and of momentum prior to either quantity being measured. But quantum mechanics considers these two observables incompatible and thus does not associate simultaneous values for both to any system. Einstein, Podolsky, and Rosen therefore concluded that quantum theory does not provide a complete description of reality.

Bell's inequalities
In 1964, Irish physicist John Stewart Bell carried the analysis of quantum entanglement much further. He deduced that if measurements are performed independently on the two separated particles of an entangled pair, then the assumption that the outcomes depend upon hidden variables within each half implies a mathematical constraint on how the outcomes on the two measurements are correlated. This constraint would later be named the Bell inequalities. Bell then showed that quantum physics predicts correlations that violate this inequality. Consequently, the only way that hidden variables could explain the predictions of quantum physics is if they are "nonlocal", which is to say that somehow the two particles are able to influence one another instantaneously no matter how widely they ever become separated.

In 1969, John Clauser and Michael Horne, along with Horne's doctoral student Abner Shimony, and Francis Pinki's doctoral student Richard Holt, came up with the CHSH inequality, a reformulation of Bell inequality that could better tested with experiments.

Early experiments in the United States
The first rudimentary experiment designed to test Bell's theorem was performed in 1972 by Clauser and Stuart Freedman at University of California, Berkeley. In 1973, at Harvard University, Pipkin and Holt's experiments suggested the opposite conclusion, negating that quantum mechanics violates the Bell inequalities. Edward S. Fry and Randall C. Thompson Texas A&M University, reattempted the experiment in 1973 and agreed with Clauser. These experiments were only a limited test, because the choice of detector settings was made before the photons had left the source.

Advised by John Bell, Alain Aspect worked to develop an experiment to remove this limitation.

In France
Alain Aspect completed his doctoral thesis in 1971 working on holography and then went abroad to teach in the École Normale in Cameroon. He returned to France in 1974 and joined the Institut d'optique in Orsay working for his habilitation thesis. Physicist Christian Imbert handled him various papers from Bell and Aspect worked for five year in the construction and preliminary tests for his experiment. He published his first experimental results in 1981, and completed his habilitation in 1983 with the final results of his experiment. The referees included André Maréchal and Christian Imbert from the Institut d'optique, Franck Laloë, Bernard d'Espagnat, Claude Cohen-Tannoudji, and John Bell.

Theoretical scheme
The illustration above represents the principle scheme from which John Bell demonstrated his inequalities: a source of entangled photons S simultaneously emits two $$\nu_1$$and $$\nu_2$$ photons whose polarization is prepared so that both photons' state vector is:


 * $$|\nu_1,\nu_2\rangle = {1 \over \sqrt{2}} \left( \left| ++\right\rangle + \left| --\right\rangle \right)$$

This formula simply means that the photons are in a superposed state: they are in a linear combination of both photons vertically polarized plus both photons horizontally polarized, with an equal probability. These two photons are then measured using two polarizers P1 and P2, each with a configurable measuring angle: α and β. the result of each polarizer's measurement can be (+) or (−) according to whether the measured polarization is parallel or perpendicular to the polarizer's angle of measurement.

One noteworthy aspect is that the polarizers imagined for this ideal experiment give a measurable result both in the (−) and (+) situations. Not all real polarizers are able to do this: some detect the (+) situation for example, but are unable to detect anything in the (−) situation (the photon never leaves the polarizer). Early experiments used the latter sort of polarizer. Alain Aspect's polarizers resulted better able to detect both scenarios and therefore much closer to the ideal experiment.

Given the apparatus and the initial state of polarization given to the photons, quantum mechanics is able to predict the probabilities of measuring (+,+), (−,−), (+,−) and (−,+) on the polarizers (P1,P2), oriented on the (α,β) angles. As a reminder in quantum mechanics:


 * $$P_{++}(\alpha,\beta) = P_{--}(\alpha,\beta) = {1 \over 2} \cos^2(\alpha-\beta)$$;


 * $$P_{+-}(\alpha,\beta) = P_{-+}(\alpha,\beta) = {1 \over 2} \sin^2(\alpha-\beta)$$.

The quantity of interest is a correlation function given by


 * $$S(\alpha,\beta;\alpha',\beta')=E(\alpha,\beta)-E(\alpha,\beta')+E(\alpha',\beta)+E(\alpha',\beta')$$

with


 * $$E(\alpha,\beta)=P_{++}(\alpha,\beta)+P_{--}(\alpha,\beta)-P_{+-}(\alpha,\beta)-P_{-+}(\alpha,\beta )$$

where (α ',β ') are a set of different angles. According to the CHSH inequality,


 * $$|S(\alpha,\beta;\alpha',\beta')|<2$$,

a type of Bell inequality. However quantum mechanics predicts a maximal violation of this inequality for |α−β| = |α' −β| = |α' −β' | = 22.5° and  |α−β' | = 67.5°.

Proposal
In 1975, since a decisive experiment based on the violation of Bell's inequalities and verifying the veracity of quantum entanglement was still missing, Alain Aspect proposed in an article, an experiment meticulous enough to be irrefutable: Proposed experiment to test the non-separability of quantum mechanics.

Alain Aspect specified his experiment so that it would be as decisive as possible. Namely:


 * Its source of entangled particles must be excellent to shorten the duration of the experiment and to provide as clear a violation of Bell's inequalities as possible.
 * It must show correlations in measurements, but also demonstrate that these correlations are indeed the result of a quantum effect (and consequently of an instantaneous influence) and not of a classical slower-than-light effect between the two particles.
 * The experimental scheme must match John Bell's as closely as possible to demonstrate his inequalities so that the agreement between the measured and predicted results be as significant as possible.

Experiments
Alain Aspect carried a three round series of increasingly complex experiments from 1980 to 1981. The first round of experiments reproduced Clauser, Holt and Fry experimental tests. In the second round of experiments he added a two-channel polarizers which improved the efficiency of the detections. These two rounds of experiments carried this experiment with the help of research engineer Gérard Roger and physicist Philippe Grangier, undergraduate student at the time.

The third round of experiments took place in 1982, and were carried in collaboration with Roger and physicist Jean Dalibard, a young student at the time. This last round is the closest to the initial specifications, will be described here.

Photon source
The first experiments testing Bell's inequalities possessed low-intensity photon sources and necessitated a continuous week to complete. One of Aspect's first improvements consisted in using a photon source several orders of magnitude more efficient. This source allowed a detection rate of 100 photons per second, thus shortening the length of the experiment to 100 seconds.

The source used is a calcium radiative cascade, excited with a krypton laser.

Polarizers with an adjustable orientation variable and on a remote position
One of the main points of this experiment was to make sure that the correlation between the measurements P1 and P2 had not been the result of "classical" effects, especially experimental artefacts.

As an example, when P1 and P2 are prepared with fixed angles α and β, it can be surmised that this state generates parasitic correlations through current or mass loops, or some other effects. As a matter of fact, both polarizers belong to the same setup and could influence one another through the various circuits of the experimental device, and generate correlations upon measurement.

One can then imagine that the fixed orientation of the polarizers impacts, one way or the other, the state the photon couple is emitted with. In such a case, the correlations between the measurement results could be explained by local hidden variables within the photons, upon their emission. Alain Aspects had mentioned these observations to John Bell himself.

One way of ruling out these kinds of effects is to determine the (α,β) orientation of the polarizers at the last moment—after the photons have been emitted, and before their detection—and to keep them far enough from each other to prevent any signal from reaching any one of them.

This method assures that the orientation of the polarizers during the emission has no bearing on the result (since the orientation is yet undetermined during emission). It also assures that the polarizers do not influence each other, being too distant from one another.

As a consequence, Aspect's experimental set-up has polarizers P1 and P2 set 6 metres apart from the source, and 12 metres apart from one another. With this setup, only 20 nanoseconds elapse between the emission of the photons and their detection. During this extremely short period of time, the experimenter has to decide on the polarizers' orientation and to then orient them.

Since it is physically impossible to modify a polarizer's orientation within such a time span, two polarizers—one for each side—were used and pre-oriented in different directions. A high-frequency shunting randomly oriented towards one polarizer or the other. The setup corresponded to one polarizer with a randomly tilting polarization angle.

Since it was not possible either to have the emitted photons provoke the tilting, the polarizers shunted periodically every 10 nanoseconds (asynchronously with the photon's emission) thus assuring the referral device would tilt at least once between the emission of the photon and its detection.

Two-channel polarizers
Another important characteristic of the 1982 experiment was the use of two-channel polarizers which allowed a measurable result in situations (+) and (−). The polarizers used until Aspect's experiment could detect situation (+), but not situation (−). These single-channel polarizers had two major inconveniences:


 * Situation (−) was difficult to discriminate from an experimentation mistake.
 * They had to be scrupulously calibrated.

The two-channel polarizers Aspect used in his experiment avoided these two inconveniences and allowed him to use Bell's formulas directly to calculate the inequalities.

Technically, the polarizers he used were polarizing cubes which transmitted one polarity and reflected the other one, emulating a Stern-Gerlach device.

Results
Bell's inequalities establish a theoretical curve of the number of correlations (++ or −−) between the two detectors in relation to the relative angle of the detectors $$(\alpha - \beta)$$. The shape of the curve is characteristic of the violation of Bell's inequalities. The measures' matching the shape of the curve establishes, quantitatively and qualitatively, that Bell's inequalities have been violated.

All three of Aspect's experiments unambiguously confirmed the violation, as predicted by quantum mechanics, thus undermining Einstein's local realistic outlook on quantum mechanics and local hidden variable scenarios. In addition to being confirmed, the violation was confirmed in the exact way predicted by quantum mechanics, with a statistical agreement of up to 242 standard deviations.

Given the technical quality of the experiment, the scrupulous avoidance of experimental artefacts, and the quasi-perfect statistical agreement, this experiment convinced the scientific community at large that quantum physics violates Bell's inequalities.

Reception and limitations
After the results, some physicists legitimately tried to look for flaws in Aspect's experiment and to find out how to improve it to resist criticism.

Some theoretical objections can be raised against the setup:


 * the quasi-periodical aspect of the shunting oscillations hinders the validity of the experiment because it can induce correlations through quasi-synchronization resulting from two referrals;
 * the correlations (+,+), (−,−) etc. were counted in real time, at the moment of detection. Each polarizer's two (+) and (−) channels were therefore linked by physical circuits. Once more, correlations may be induced.

The ideal experiment, which would negate any imaginable possibility of induced correlations should:


 * use purely random shunting;
 * record the (+) or (−) results on each side of the device, without any physical link between the two sides. The correlations would be calculated after the experiment, by comparing the recorded results of both sides.

The conditions of the experiment also suffered from a detection loophole.

After 1982, physicists began to look for application of entanglement, this lead for the development of quantum computing and quantum cryptography.

For his work on this topic, Aspect received several awards including the 2010 Wolf Prize in Physics and the 2022 Nobel Prize in Physics, both shared with John Clauser and Anton Zeilinger for their Bell tests.

Later experiments
The loopholes mentioned could only be solved from 1998. In the meantime, Aspect's experiment was reproduced, and the violation of Bell's inequalities was systematically confirmed, with a statistical certainty of up to 100 standard deviation.

Other experiments were conducted to test the violations of Bell's inequalities with other observables than polarization, in order to approach the original spirit of the EPR paradox, in which Einstein imagined measuring two combined variables (such as position and movement quantity) on an EPR pair. An experiment introduced the combined variables (time and energy) which, once again, confirmed quantum mechanics.

In 1998, the Geneva experiment tested the correlation between two detectors set 30 kilometres apart using the Swiss optical fibre telecommunication network. The distance gave more time to commute the angles of the polarizers. It was therefore possible to have a completely random shunting. Additionally, the two distant polarizers were entirely independent. The measurements were recorded on each side, and compared after the experiment by dating each measurement using an atomic clock. The violation of Bell's inequalities was once again verified under strict and practically ideal conditions. If Aspect's experiment implied that a hypothetical coordination signal travel twice as fast as the speed of light c, Geneva's reached 10 million times c.

An experiment took place at the National Institute of Standards and Technology (NIST) in 2000 on trapped-ion entanglement using a very efficient correlation-based detection method. The reliability of detection proved to be sufficient for the experiment to violate Bell's inequalities on the whole, even though all detected correlations did not violate them.

In 2001, Antoine Suarez's team, which included Nicolas Gisin who had participated in the Geneva experiment, reproduced the experiment using mirrors or detectors in motion, allowing them to reverse the order of events across the frames of reference, in accordance with special relativity (this inversion is only possible for events without any causal relationship). The speeds are chosen so that when a photon is reflected or crosses the semi-transparent mirror, the other photon has already crossed or been reflected from the point of view of the frame of reference attached to the mirror. This an "after-after" configuration, in which sound waves play the role of semi-transparent mirrors.

In 2015 the first three significant-loophole-free Bell-tests were published within three months by independent groups in Delft University of Technology, University of Vienna and NIST. All three tests simultaneously addressed the detection loophole, the locality loophole, and the memory loophole.

Implications
Prior to the Aspect experiments, Bell's theorem was mostly a niche topic. The publications by Aspect and collaborators prompted wider discussion of the subject.

The fact that nature is found to violate Bell's inequality implies that one or more of the assumptions underlying that inequality must not hold true. Different interpretations of quantum mechanics provide different views on which assumptions ought to be rejected. Copenhagen-type interpretations generally take the violation of Bell inequalities as grounds to reject the assumption often called counterfactual definiteness. This is also the route taken by interpretations that descend from the Copenhagen tradition, such as consistent histories (often advertised as "Copenhagen done right"), as well as QBism. In contrast, the versions of the many-worlds interpretation all violate an implicit assumption by Bell that measurements have a single outcome. Unlike all of these, the Bohmian or "pilot wave" interpretation abandons the assumption of locality: instantaneous communication can exist at the level of the hidden variables, but it cannot be used to send signals.